Selected publications:

The Detection of Monoclinic Zirconia and Non-Uniform 3D Crystallographic Strain in a Re-Oxidized Ni-YSZ Solid Oxide Fuel Cell Anode.Thomas M. M. Heenan, Antonis Vamvakeros, Chun Tan, Donal P. Finegan, Sohrab R. Daemi, Simon D. M. Jacques, Andrew M. Beale, Marco Di Michiel, Dan J. L. Brett and Paul R. Shearing, Crystals 2020, 10, 941., https://doi.org/10.3390/cryst10100941

Exploring cycling induced crystallographic change in NMC with X-ray diffraction computed tomography. Sohrab R. Daemi,  Chun Tan,  Antonis Vamvakeros, Thomas M. M. Heenan,  Donal P. Finegan,   Marco Di Michiel,  Andrew M. Beale,  James Cookson,  Enrico Petrucco,  Julia S. Weaving,  Simon Jacques, Rhodri Jervis, Dan J. L. Brett  and  Paul R. Shearing, Phys. Chem. Chem. Phys., 2020,22, 17814-17823, https://doi.org/10.1039/D0CP01851A

Real-time tomographic diffraction imaging of catalytic membrane reactors for the oxidative coupling of methane. Antonis VamvakerosDorota MatrasSimon D.M. Jacques, Marcodi Michiel, Vesna Middelkoop, Peixi Cong, Stephen W.T. Price, Craig L. Bull, Pierre Senecal, Andrew M. Beale, Catalysis Today, Available online 19 May 2020, Advance Article, https://doi.org/10.1016/j.cattod.2020.05.045

In situ X-ray diffraction computed tomography studies examining the thermal and chemical stabilities of working Ba0.5Sr0.5Co0.8Fe0.2O3−δmembranes during oxidative coupling of methane. Dorota Matras, Antonis Vamvakeros,  Simon D. M. Jacques, Vesna Middelkoop,  Gavin Vaughan,  Miren Agote Aran,    Robert J. Cernik  and  Andrew M. Beale, Phys. Chem. Chem. Phys., June 2020, Advance Article, https://doi.org/10.1039/D0CP02144J

Exploring cycling induced crystallographic change in NMC with X-ray diffraction computed tomography. Sohrab R. Daemi,  Chun Tan,   Antonis Vamvakeros,  Thomas M. M. Heenan,  Donal P. Finegan,  Marco Di Michiel,  Andrew M. Beale,  James Cookson, Enrico Petrucco,  Julia S. Weaving,   Simon Jacques,  Rhodri Jervis, Dan J. L. Brett  and  Paul R. Shearing, Phys. Chem. Chem. Phys., June 2020, Advance Article,    https://doi.org/10.1039/D0CP01851A

In Situ Study of Graphene Oxide Quantum Dot-MoSx Nanohybrids as Hydrogen Evolution Catalysts. Marco Favaro, Mattia Cattelan, Stephen W. T. Price, Andrea E. Russell, Laura Calvillo, Stefano Agnoli and Gaetano Granozzi, Surface Science and Catalysis of Graphene-Related 2D Materials, 16 June 2020, Surfaces, 3(2), 225-236; https://doi.org/10.3390/surfaces3020017

Real-time multi-length scale chemical tomography of fixed bed reactors during the oxidative coupling of methane reaction. Antonis VamvakerosDorota MatrasSimon D.M. Jacques, Marco di Michiel, Stephen W.T. Price, Pierre Senecal, Miren Agote Aran, Vesna Middelkoop, Gavin B.G. Stenning, J. Frederick W. Mosselmans, Ilyas Z. Ismagilov & Andrew M. Beale. Journal of Catalysis, Volume 386, June 2020, Pages 39-52. DOI: https://doi.org/10.1016/j.jcat.2020.03.027

Effect of thermal treatment on the stability of Na-Mn-W/SiO2 Catalyst for the Oxidative Coupling of Methane.

Spatial quantification of dynamic inter and intra particle crystallographic heterogeneities within lithium ion electrodes. Finegan, D.P., Vamvakeros, A., Tan, C, Chun Tan, Thomas M. M. Heenan, Sohrab R. Daemi, Natalie Seitzman, Marco Di Michiel, Simon Jacques, Andrew M. Beale, Dan J. L. Brett, Paul R. Shearing & Kandler Smith,  Nat Commun 11, 631 (2020). https://doi.org/10.1038/s41467-020-14467-x

Sustainable iron-based oxygen carriers for hydrogen production – Real-time operando investigation. Yoran De Vos, Antonis Vamvakeros, Dorota Matras, Marijke Jacobs, Pascal Van Der Voort, Isabel Van Driessche, Simon Jacques, Vesna Middelkoop, AnVerberckmoes, International Journal of Greenhouse Gas Control, Volume 88, September 2019, Pages 393-402, https://doi.org/10.1016/j.ijggc.2019.06.016

3D printed Ni/Al2O3 based catalysts for CO2methanation – a comparative and operando XRD-CT study, Vesna Middelkoop, AntonisVamvakeros, Dieterde Wit, Simon D.M. Jacques, Simge Danaci, Clement Jacquot, Yorande Vos, Dorota Matras, Stephen W.T.Price, Andrew M.Beale, Journal of CO2 Utilization, Volume 33, October 2019, Pages 478-487, https://doi.org/10.1016/j.jcou.2019.07.013

Spatially Resolving Lithiation in Silicon–Graphite Composite Electrodes via in Situ High-Energy X-ray Diffraction Computed Tomography. Donal P. Finegan, Antonis Vamvakeros, Lei Cao, Chun Tan, Thomas M. M. Heenan, Sohrab R. Daemi, Simon D. M. Jacques, Andrew M. Beale, Marco Di Michiel, Kandler Smith, Dan J. L. Brett, Paul R. Shearing and Chunmei Ban, Nano Lett.2019, https://doi.org/10.1021/acs.nanolett.9b00955

Design of next-generation ceramic fuel cells and real-time characterization with synchrotron X-ray diffraction computed tomography. Tao Li, Thomas M. M. Heenan, Mohamad F. Rabuni, Bo Wang, Nicholas M. Farandos, Geoff H. Kelsall, Dorota Matras, Chun Tan, Xuekun Lu, Simon D. M. Jacques, Dan J. L. Brett, Paul R. Shearing, Marco Di Michiel, Andrew M. Beale, Antonis Vamvakeros & Kang Li, Nature Communications, volume 10, Article number: 1497 (2019), DOI: https://doi.org/10.1038/s41467-019-09427-z

Operando and Post-Reaction Diffraction Imaging of La-Sr/CaO Catalyst in the Oxidative Coupling of Methane Reaction. D. Matras, S. D. M. Jacques, S. Poulston, N. Grosjean, C. Estruch Bosch, B. Rollins, J. Paul Wright, M. Di Michiel, A. Vamvakeros, R. J. Cernik, and A. M. Beale. J. Phys. Chem. C, January 2, 2019 (web), 123, 1751–1760.

Unravelling the spatial dependency of the complex solid-state chemistry of Pb in a paint micro-sample from Rembrandt’s Homer using XRD-CT. Stephen W T Price, Annelies Van Loon, Katrien Keune, Aaron Parsons, Claire Murray, Andrew M Beale, J Fred W Mosselmans. Chemical Communications, 2019, DOI: 10.1039/C8CC09705D

5D operando tomographic diffraction imaging of a catalyst bed. A. Vamvakeros, S. D. M. Jacques, M. Di Michiel, D. Matras, V. Middelkoop, I. Z. Ismagilov, E. V. Matus, V. V. Kuznetsov, J. Drnec, P. Senecal & A. M. Beale. (2018). Nature Communications, volume 9, Article number: 4751

Real-Time Operando Diffraction Imaging of La-Sr/CaO During the Oxidative Coupling of Methane. Matras, D. Jacques, S. D. M. Godini, H. R. Khadivi, M. Drnec, J. Poulain, A. Cernik, R. J.Beale, A. M. J. Phys. Chem. C, 2018, 122, 2221-2230.

Chemical imaging of Fischer-Tropsch catalysts under operating conditions. Price, S. W. T., Martin, D. J., Parsons, A. D., Sławiński, W. A., Vamvakeros, A., Keylock, S. J., . . . Mosselmans, J. F. W. (2017). Science Advances, 3 (3), e1602838.

Real-Time Scattering-Contrast Imaging of a Supported Cobalt-Based Catalyst Body during Activation and Fischer-Tropsch Synthesis Revealing Spatial Dependence of Particle Size and Phase on Catalytic Properties. Senecal, P., Jacques, S. D. M., Di Michiel, M., Kimber, S. A. J., Vamvakeros, A., Odarchenko, Y., . . . Beale, A. M. (2017). ACS Catalysis, 7 (4), 2284

Reversible restructuring of supported Au nanoparticles during butadiene hydrogenation revealed by operando. GISAXS/GIWAXS. Martin, D. J., Decarolis, D., Odarchenko, Y. I., Herbert, J. J., Arnold, T., Rawle, J., . . . Beale, A. M. (2017) Chem Comm, 53 (37), 5159-5162.

Molybdenum Speciation and its Impact on Catalytic Activity during Methane Dehydroaromatization in Zeolite ZSM-5 as Revealed by Operando X-Ray Methods. Lezcano-González, I., Oord, R., Rovezzi, M., Glatzel, P., Botchway, S. W., Weckhuysen, B. M., & Beale, A. M. (2016) Ange. Chemie Int. Ed., 55 (17), 5348.

Interlaced X-ray diffraction computed tomography A. Vamvakeros, S.D.M. Jacques, M. Di Michiel, P. Senecal, V. Middelkoop, R.J. Cernik and A.M. Beale. Journal of Applied Crystallography (2016) 49, 485.

Removing multiple outliers and single-crystal artefacts from X-ray diffraction computed tomography data A. Vamvakeros, S.D M. Jacques, M. Di Michiel, V. Middelkoop, C. K. Egan, R. J. Cernik and A.M. Beale. Journal of Applied Crystallography (2015) 48, 1943

3D chemical imaging in the laboratory by hyperspectral X-ray computed tomography. C.K. Egan, S.D.M. Jacques, M.D. Wilson, M.C. Veale, P. Seller, A.M. Beale, R.A.D. Pattrick, P.J. Withers & R.J. Cernik. Scientific Reports (2015) 5, 15979

Real time chemical imaging of a working catalytic membrane reactor during oxidative coupling of methane. A. Vamvakeros, S.D.M. Jacques, V. Middelkoop, M. Di Michiel, C.K. Egan, I.Z. Ismagilov, G.B.M. Vaughan, F. Gallucci, M. van Sint Annaland, P.R. Shearing, R.J. Cernik and A.M. Beale. Chem. Commun. (2015) 51, 12752

Progress towards Five Dimensional Imaging of Functional Materials Under Process Conditions. A.M. Beale, S.D.M. Jacques, E.K. Gibson and M Di Michiel. Coordination Chemistry Reviews (2014) 277-278, 208

Chemical imaging of sulphur-induced deactivation of Cu/ZnO catalyst bodies. A.M. Beale, E.K. Gibson, M.G. O’Brien, S.D.M. Jacques, R.J. Cernik, M. Di Michiel, P.D. Cobden, Ö. Pirgon-Galin, L. de Water, M. J Watson, and B. M. Weckhuysen. J. Catalysis (2014) 314, 94.

Imaging the Continuous Hydrothermal Flow Synthesis of Nanoparticulate CeO2 at Different Supercritical Water Temperatures Using in Situ Angle-Dispersive Diffraction. V. Middelkoop, C.J. Tighe, S. Kellici, S.D.M. Jacques, J.M. Perkins, R.I. Gruar, P. Barnes and J.A. Darr. J. Supercritical Fluids (2014) 87, 118-128

Pair distribution function computed tomography. S.D.M. Jacques, M. Di Michiel, S.A.J. Kimber, X. Yang, R.J. Cernik, S.J.L. Billinge and A.M. Beale. Nat. Comm. (2013) 4, 2536.

Active phase evolution in single Ni/Al2O3 methanation catalyst bodies studied in real time using combined μ -XRD-CT and μ-absorption-CT. M.G. O’Brien, S.D.M. Jacques, M. Di Michiel, P. Barnes, B.M. Weckhuysen and A.M. Beale, Chem. Sci., 3 (2012) 509-523.

Chemical Probing within Catalyst Bodies by Diagonal Offset Raman Spectroscopy. M.W. Zandbergen, S.D.M. Jacques, B.M. Weckhuysen and A.M. Beale, Angewandte Chemie-Int. Ed., 51 (2012) 957-960.

Dynamic X-ray diffraction computed tomography reveals real-time insight into catalyst active phase evolution. S.D.M. Jacques, M. Di Michiel, A. M. Beale, T. Sochi, M. G. O’Brien, L. Espinosa-Alonso, B. M. Weckhuysen and P. Barnes, Angewandte Chemie-Int. Ed., 50, (2011), 10148-10152